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- W2014808618 abstract "We summarize and discuss some of the available experimental and theoretical data important for understanding the role played by subsurface sites in dissociative chemisorption calculations for the H2/Pd(111) system. Then we use a semi-empirical potential energy surface (PES) to model the interaction of a H2 molecule impinging on a Pd(111) surface. The London–Eyring–Polanyi–Sato (LEPS) construction has been extended to make direct subsurface absorption possible. A two-dimensional wave packet calculation is used to find qualitative trends in the direct subsurface absorption and to reveal the time scales involved. We suggest that a partial in-plane relaxation occurs for the slowest incoming particles, thus resulting in a higher direct subsurface absorption probability for low energies." @default.
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- W2014808618 title "Direct subsurface absorption of hydrogen on Pd(111)" @default.
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- W2014808618 doi "https://doi.org/10.1063/1.471541" @default.
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