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- W2014869847 abstract "No reliable rate constant is available for the self-reaction of tert-;butoxy radicals. We have set up a competition between hydrogen abstraction and self-reaction of tert-butoxy radicals in a flash photolysis electron spin resonance study to extract this information. Experimental values of hydrogen abstraction product radical concentrations under various hydrogen donor concentrations were then compared with theoretically calculated values with different values of 2k4 to obtain the best fit. Hydrogen donors such as cyclopentane, anisole, methyl tert-butyl ether, and methanol were chosen for the study. A value of (1.3 ± 0.5) × 109M−1 sec−1 for the rate constant of the self-reaction of tert-butoxy radicals has been determined at 293°K." @default.
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- W2014869847 date "1981-05-01" @default.
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- W2014869847 title "An indirect measurement of the absolute rate constant of the self-reaction oftert-butoxy radicals" @default.
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- W2014869847 doi "https://doi.org/10.1002/kin.550130502" @default.
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