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• W2014960983 abstract "Polarized and depolarized dynamic light scattering have been used to examine the dynamics of concentrated polystyrene solutions in dioctyl phthalate and toluene. Time-temperature superposition of the depolarized intensity correlation functions gave master curves covering more than 10 decades on the time scale. Polarized correlation functions are resolved into relaxational and diffusive components having different temperature dependences. When the relaxation rate of the concentration fluctuations approaches the reorientational relaxation rate, the concentration fluctuations become q-independent i.e. the diffusional relaxation is rate-determined by the backbone mobility. With a small molecule solvent as toluene, however, a part of the concentration fluctuations relaxes faster than the orientational relaxation, i.e., the diffusion occurs in the free volume within the “frozen” network." @default.
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• W2014960983 date "1994-03-01" @default.
• W2014960983 modified "2023-10-02" @default.
• W2014960983 title "Polarized and depolarized dynamic light scattering of concentrated polystyrene solutions" @default.
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• W2014960983 doi "https://doi.org/10.1002/masy.19940790114" @default.
• W2014960983 hasPublicationYear "1994" @default.
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