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- W2014963493 abstract "A very simple (semiclassical) treatment of nonreactive atom—diatom collisions permits the analytic approximation of inelastic state to state scattering cross sections. The derived energy dependence of these cross sections is found to be reasonably independent of the form of the effective (model) scattering potential indicating some generality of applicability. These results provide a generalization of the familiar (empirical) linear surprisal (exponential gap) relationship encountered in vibrationally or rotationally inelastic scattering. Explicit expressions are given for the surprisal parameters of Levine and Bernstein et al. These are evaluated for several rotationally inelastic processes. The theory is seen to predict correctly the observed surprisal slopes and their energy and mass dependence. It also predicts deviations from the linear surprisal from when states having high internal energies are involved. For the more complex case of both vibrationally and rotationally inelastic scattering certain simple behavior of the surprisals (inelastic cross sections) is expected in limiting energy regions. We suggest that linear surprisals will not be general for systems which do not conform to the model assumptions. We conclude that linear surprisals are manifestations of scattering processes which are dominated by the translational dynamics. The surprisal slope measures the range of the effective scattering potential. The details of the potential surface therefore are relatively unimportant." @default.
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- W2014963493 date "1977-01-01" @default.
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- W2014963493 title "Exponential gap law for atom—diatom inelastic scattering" @default.
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- W2014963493 doi "https://doi.org/10.1016/0009-2614(77)85210-x" @default.
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