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- W2015173817 abstract "Pillared interlayer clays (PILCs) were synthesized by pillaring montmorillonite with SiO2, Al2O3, and ZrO2, and Co-supported PILCs were prepared by the impregnation method. For comparison, Co/SiO2 and Co-supported montmorillonite treated with dilute HNO3 (acid-clay) were also prepared. The materials were characterized by XRD, H2-TPR, NH3-TPD, O2 titration, and N2 adsorption−desorption. The Co-supported catalysts were comparatively investigated for Fischer−Tropsch (FT) synthesis in a fixed-bed reactor under the conditions of 1 MPa, 508 K, H2/CO = 2, and W/F = 5.02 g·h·mol−1. The results indicate that the activities of the catalysts (i.e., CO conversions) increase in the order of Co/Na-Clay ≪ Co/Si-PILC ≈ Co/acid-clay ≈ Co/Al-PILC < Co/Zr-PILC ≈ Co/SiO2. Moreover, Co/PILCs can effectively narrow the product distribution of FT synthesis showing significantly increased C5−C12 selectivity and much decreased C21+ selectivity. The results are well explained based on the acidic properties of the PILCs together with the textural properties, pore size distributions, and reduction behaviors of the catalysts." @default.
- W2015173817 created "2016-06-24" @default.
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- W2015173817 date "2010-08-30" @default.
- W2015173817 modified "2023-09-26" @default.
- W2015173817 title "Co/Pillared Clay Bifunctional Catalyst for Controlling the Product Distribution of Fischer−Tropsch Synthesis" @default.
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- W2015173817 doi "https://doi.org/10.1021/ie101163w" @default.
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