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- W2015188001 abstract "Abstract The kinetics of H(D) absorption into a β-phase PdH x (PdD x ) electrode are discussed numerically, based on the Volmer–Tafel route of the hydrogen (deuterium) evolution reaction and thermodynamic and kinetic data of H(D) in the β-phase PdH x (PdD x ). It is found that the asymptotic loading ratio of H(D) is determined only by the Tafel step under galvanostatic conditions. The kinetics of H(D) absorption can be characterised by a parameter λ ∝ d Δ j /( D Δ x ) where d is the dimension of the electrode (thickness for plate, radii for cylinder or sphere); Δ j is the current density step; D is the average diffusion coefficient; Δ x is the loading ratio step of H(D) caused by the current step. If λ ⪢1 (large scale of dimension, high current density and/or low temperature), the absorption rate is controlled by diffusion; in contrast, if λ ≪1, the rate-determining step is the interface process and the charging efficiency approaches 100%; otherwise, the kinetics are under mixed control if λ ∼1." @default.
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- W2015188001 date "1999-09-01" @default.
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- W2015188001 title "Numerical simulation of hydrogen (deuterium) absorption into β-phase hydride (deuteride) palladium electrodes under galvanostatic conditions" @default.
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- W2015188001 doi "https://doi.org/10.1016/s0022-0728(99)00349-6" @default.
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