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• W2015225849 endingPage "1062" @default.
• W2015225849 startingPage "1053" @default.
• W2015225849 abstract "In this paper the impact of peripheral substitution with a strongly withdrawing fused ring group on the optical spectroscopy of a metal phthalocyanine complex is analyzed. We report the synthesis of [9 (or 10), 16 (or 17), 23 (or 24)-tri-tert-butylimidophthalocyaninato]zinc(II) (ZnttbIPc), which should eventually prove to be a useful precursor for forming dimeric compounds. The electronic structure is analyzed through a detailed analysis of the UV-visible absorption and magnetic circular dichroism spectra and time-dependent density functional theory calculations. Other than a marked splitting of the Q band, the spectrum is broadly similar to that of ZnPc in terms of the main π → π* electronic bands. The vibrational bands differ markedly in the Q band region when an imido group is added to ligand periphery, relative to what is observed in the case of zinc mononaphthotribenzotetraazaporphyrin ( Zn3B1N ) with an additional fused benzene ring. The absorption and emission spectra lack mirror symmetry as is the case with ZnPc and thus provide possible evidence for a second set of electronic origins in the Q band region arising from n → π* rather then π → π* transitions." @default.
• W2015225849 created "2016-06-24" @default.
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• W2015225849 date "2009-10-01" @default.
• W2015225849 modified "2023-10-14" @default.
• W2015225849 title "Effect of peripheral fused ring substitution on the optical spectroscopy and electronic structure of metal phthalocyanine complexes" @default.
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• W2015225849 doi "https://doi.org/10.1142/s1088424609001339" @default.
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