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• W2015271461 abstract "The partial oxidation of methanol to formaldehyde on ceria-supported monolayer vanadium oxide was studied using temperature-programmed desorption (TPD), microcalorimetry, and X-ray photoelectron spectroscopy (XPS). Methanol TPD demonstrated that the activation energy for the dehydrogenation of adsorbed methoxides to produce formaldehyde is a function of the oxidation state of the vanadium cations in the supported layer. During CH3OH TPD, CH2O was produced at 525, 550, and 610 K, on V5+, V4+, and V3+, respectively. The heat of reoxidation of supported vanadia/ceria samples that had been reduced by performing a CH3OH TPD experiment was measured using microcalorimetry and found to be 245 kJ/mol of O2. The heat of adsorption of CH3OH on the vanadia layer was also measured and found to be 80 kJ/mol on both oxidized and partially reduced VOx/CeO2 samples. The implications of these results for understanding the mechanism of methanol oxidation on supported vanadia are discussed." @default.
• W2015271461 created "2016-06-24" @default.
• W2015271461 creator A5003605373 @default.
• W2015271461 creator A5081810695 @default.
• W2015271461 date "2004-01-25" @default.
• W2015271461 modified "2023-09-29" @default.
• W2015271461 title "A TPD study of the partial oxidation of methanol to formaldehyde on CeO2-supported vanadium oxide" @default.
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• W2015271461 doi "https://doi.org/10.1016/j.jcat.2003.10.002" @default.
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