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• W2015295093 abstract "Using a recently-developed chemiluminescence technique for monitoring O(1D), the rate coefficient, k1, of the important atmospheric reaction O(1D) + CH4 --> products has been determined over a wide temperature range, 227 to 450 K. The rate coefficient was shown to be independent of temperature, having a value of (1.91 +/- 0.08) x 10(-10) cm3 s(-1); the quoted uncertainties are with 95% confidence. This highly precise value, based on an extended set of determinations with very low scatter, is significantly greater, 26%, than current recommended values. Secondly, the fraction of O(1D) quenched to O(3P) by CH4, k(1q)/k1, was precisely determined from chemiluminescence decays over the temperature range 236 to 340 K. A temperature independent value for k(1q)/k1 of 0.002 +/- 0.003 was found. Finally, LIF detection of OH has been applied to accurately determine the product branching fraction to OH of O(1D) + CH4 at room temperature. Our value, k(1a)/k1 = 0.76 +/- 0.08 (95% confidence), is in line with recent determinations by other groups." @default.
• W2015295093 created "2016-06-24" @default.
• W2015295093 creator A5045737008 @default.
• W2015295093 creator A5083491990 @default.
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• W2015295093 date "2008-01-01" @default.
• W2015295093 modified "2023-09-26" @default.
• W2015295093 title "A temperature dependence kinetic study of O(1D) + CH4: overall rate coefficient and product yields" @default.
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• W2015295093 doi "https://doi.org/10.1039/b804903c" @default.
• W2015295093 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/18956106" @default.
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