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- W2015306596 abstract "Abstract Electron spin resonance (ESR) studies have been carried out on the layered copper oxycarbonates (alternating layers of CuO2 and CO2-3) with the nominal composition Ba3SrCu2O6.2CO2 and their reaction products with ammonium slats. The ESR signals typical of copper ions in square-planar geometry with a slight orthorhombic distortion presumably arise from the copper ions being incorporated in the carbonate layer. A simple grinding procedure at room temperature using (NH+4)nXn- (X=F-, (NO3)-, (VO3)-, (HPO4)2-) incorporates Xn- anions in the structure with the liberation of ammonia. The environment of the cop per ion in the carbonate layer is thus changed without altering the structure. The g3 values are most affected by this reaction showing that the filled eg orbitals are oriented in the plane of the carbonate layer. The half-filled eg orbitals (transforming s dx2−y2 orbitals) are oriented out of the plane. This suggests that the copper ions in the carbonate layers are probably involved in introducing magnetic coupling between the CuO2 layers." @default.
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- W2015306596 date "1993-02-01" @default.
- W2015306596 modified "2023-10-02" @default.
- W2015306596 title "Electron spin resonance evidence for the role of copper ions in interlayer coupling in layered copper oxycarbonates" @default.
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- W2015306596 doi "https://doi.org/10.1016/0921-4534(93)90702-r" @default.
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