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- W2015452287 abstract "New coordination environments are reported for Np(iii) and Pu(iii) based on pilot studies of U(iii) in 2.2.2-cryptand (crypt). The U(iii)-in-crypt complex, [U(crypt)I2][I], obtained from the reaction between UI3 and crypt, is treated with Me3SiOTf (OTf = O3SCF3) in benzene to form the [U(crypt)(OTf)2][OTf] complex. Similarly, the isomorphous Np(iii) and Pu(iii) complexes were obtained similarly starting from [AnI3(THF)4]. All three complexes (1-An; An = U, Np, Pu) contain an encapsulated actinide in a THF-soluble complex. Absorption spectroscopy and DFT calculations are consistent with 5f3 U(iii), 5f4 Np(iii), and 5f5 Pu(iii) electron configurations." @default.
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- W2015452287 date "1979-01-01" @default.
- W2015452287 modified "2023-10-17" @default.
- W2015452287 title "Behaviour of uranium (VI) with some cryptands in aqueous solution" @default.
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- W2015452287 doi "https://doi.org/10.1016/0020-1650(79)80119-1" @default.
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