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• W2015618635 startingPage "995" @default.
• W2015618635 abstract "Nitrogen dioxide (NO 2 ) and nitric acid (HNO 3 ) distributions were derived with a two‐dimensional time‐dependent model using N 2 O, CH 4 , and temperature measurements from the stratospheric and mesospheric sounder (SAMS) along with H 2 O measurements from the limb infrared monitor of the stratosphere (LIMS) and O 3 measurements from the solar backscatter ultraviolet (SBUV) instrument. All three instruments (SAMS, LIMS, and SBUV) were aboard the Nimbus 7 satellite. The computed NO 2 and HNO 3 were compared with LIMS NO 2 and HNO 3 measurements. Calculated NO 2 is lower than the LIMS NO 2 in much of the lower stratosphere by about a factor of 4 or more. Differences in the upper stratosphere between derived NO 2 and LIMS NO 2 are within the photochemical uncertainties of the computation. Derived NO 2 is much larger than LIMS NO 2 at high latitudes in the upper stratosphere in December, indicating that dynamics and/or photochemistry in the atmosphere are different from those used in the model. Derived HNO 3 is in fairly good agreement with LIMS HNO 3 in the upper stratosphere. Derived and LIMS HNO 3 gradually become more different through the middle stratosphere and reach a fairly substantial disagreement in the lower stratosphere. The high‐latitude maxima observed in LIMS HNO 3 are present at lower altitudes and at higher concentrations than those derived in the model computations. More significantly, the derived HNO 3 at polar latitudes is highest in the summer while LIMS HNO 3 is highest in the winter. Disagreements in the lower stratosphere between the computed and LIMS NO 2 and HNO 3 can only be reduced if two changes are made in the model computations: (1) additional lower stratospheric sources of odd nitrogen (other than N 2 O + O( 1 D )) are included and (2) a modified chemistry to allow the formation of HNO 3 at the expense of N 2 O 5 is used." @default.
• W2015618635 created "2016-06-24" @default.
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• W2015618635 date "1987-01-20" @default.
• W2015618635 modified "2023-10-08" @default.
• W2015618635 title "An intercomparison of nitrogen‐containing species in Nimbus 7 LIMS and SAMS data" @default.
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• W2015618635 doi "https://doi.org/10.1029/jd092id01p00995" @default.
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