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- W2015655004 abstract "We have studied spin–orbit perturbations between the A(2) 1Σ+ and b(1) 3Π0 states of the NaK molecule by accurately measuring the energies of mutually perturbing levels, and by measuring ratios of A(2) 1Σ+ → X(1) 1Σ+ and b(1) 3Π0 → a(1) 3Σ+ emission intensities, for five perturbed pairs. This allows two partially independent determinations of each perturbation matrix element ‖〈1 3Π0(v′t, J′)‖Ĥso‖21Σ+(v′s,J′)〉‖. From these matrix elements, and calculated vibrational overlap integrals 〈v′t‖v′s〉, the electronic part of the perturbation matrix element, Hel≡‖〈1 3Π0(v′t, J′)‖Ĥso‖2 1Σ+(v′s, J′)〉‖/‖〈v′t‖v′s〉‖, was obtained. Our results for Hel from the two methods are consistent, and independent of vibrational and rotational quantum numbers, as expected. The determined best value for Hel is (15.64±0.39) cm−1." @default.
- W2015655004 created "2016-06-24" @default.
- W2015655004 creator A5020872234 @default.
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- W2015655004 date "1992-10-01" @default.
- W2015655004 modified "2023-09-25" @default.
- W2015655004 title "Spin–orbit perturbations between the <i>A</i>(2)1Σ+ and <i>b</i>(1)3Π states of NaK" @default.
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- W2015655004 doi "https://doi.org/10.1063/1.463990" @default.
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