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- W2015656377 abstract "Until the work of Trost and Schroeder (J. Am. Chem. Soc. 1999, 121, 6759), transition-metal-catalyzed asymmetric allylic alkylation (AAA) reactions were confined to the use of ‘soft’, stabilized carbanions. However, general methods to apply carboxylic acid carbanions in AAA reactions remain undeveloped. As a large step forward, the authors report the use of acyclic amides as nucleophiles in the Pd-catalyzed AAA reaction with 1,1′-P,N ferrocene ligand L1. Alkylation of a variety of α-substituted aliphatic and aromatic amides proceeded in high yield with good to high levels of asymmetric induction." @default.
- W2015656377 created "2016-06-24" @default.
- W2015656377 date "2008-04-23" @default.
- W2015656377 modified "2023-10-17" @default.
- W2015656377 title "Asymmetric Allylic Alkylation with ‘Hard’ Amide Carbanions" @default.
- W2015656377 doi "https://doi.org/10.1055/s-2008-1072636" @default.
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