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- W2015854433 abstract "Ultrafast vibrational dynamics of hydrogen bond network at the air/water interface is revealed by two-dimensional heterodyne-detected vibrational sum frequency generation (2D HD-VSFG) spectroscopy. Three diagonal peaks are clearly observed in the 2D HD-VSFG spectrum, which correspond to the negative and positive hydrogen-bonded OH stretch bands and the positive “free” OH stretch band in the steady-state HD-VSFG spectrum. A diagonally elongated bleaching lobe of the hydrogen-bonded OH at 0 ps indicates that it is partly inhomogeneously broadened. This diagonal elongation vanishes in a few hundred femtoseconds, implying the ultrafast spectral diffusion in the hydrogen-bonded OH band. Off-diagonal cross peaks between each OH oscillator are clearly observed instantaneously within the time resolution of 0.2 ps, suggesting that they are vibrationally coupled through anharmonicity and/or energy transfer." @default.
- W2015854433 created "2016-06-24" @default.
- W2015854433 creator A5023702917 @default.
- W2015854433 date "2013-10-22" @default.
- W2015854433 modified "2023-10-18" @default.
- W2015854433 title "Communication: Ultrafast vibrational dynamics of hydrogen bond network terminated at the air/water interface: A two-dimensional heterodyne-detected vibrational sum frequency generation study" @default.
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- W2015854433 doi "https://doi.org/10.1063/1.4826095" @default.
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