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• W2016022612 abstract "The reaction of metastable Ar(3P0,2) atoms with PCl3 has been developed as a source of metastable PCl(b1Σ+) molecules in a flow reactor at 300 K. The total quenching rate constants were measured for 23 molecules, and they are in the 2 × 10-14 to 3 × 10-11 cm3 molecule-1 s-1 range. An electronic-to-vibrational (E−V) energy-transfer mechanism is used to discuss the quenching of PCl(b1Σ+), and the experimental rate constants are compared to similar data for PF(b1Σ+), NF(b1Σ+), and NCl(b1Σ+) molecules. An influence of the type of halogen substituent in the reagent molecule on the quenching rate constants is identified, and a role for attractive molecular interactions needs to be added to the E−V model. The Ar(3P0,2) + PCl3 reaction gives vibrationally excited PCl(b1Σ+) molecules and the Δv = +1 and +2 sequences were observed in addition to the Δv = 0 main sequence." @default.
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• W2016022612 date "1997-10-01" @default.
• W2016022612 modified "2023-09-22" @default.
• W2016022612 title "Quenching Rate Constants for PCl(bΣ⁺, <i>v</i>‘ = 0)" @default.
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• W2016022612 doi "https://doi.org/10.1021/jp971031s" @default.
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