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- W2016058138 abstract "Carbon-supported Pd-rich pseudo-core-shell Pd-Pt (Pd@Pt/C) nanoparticles, with Pt coverage close to a monolayer, were prepared from a simple galvanic replacement reaction between Pd/C particles and PtCl 2- 4 at 100°C. The pseudo-core-shell architecture was confirmed by extensive microstructural characterization techniques. The binding energy shifts in the Pt 4f X-ray photoelectron spectra, in particular, suggest an electron exchange between Pd and Pt, and possible strain effects in Pt caused by the underlying Pd core. The activity of the pseudo-core-shell nanoparticles in the oxygen reduction reaction (ORR) was studied in acidic solutions with and without methanol. The electrocatalysts prepared as such were active for ORR at room temperature, even in the presence of 0.1 M methanol. The pseudo-core-shell Pd 70 @Pt 30 catalyst, in particular, compared rather favorably with a Pt/C catalyst with twice the Pt mass loading in terms of the ORR activity, cost, and methanol tolerance." @default.
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- W2016058138 date "2008-01-01" @default.
- W2016058138 modified "2023-09-26" @default.
- W2016058138 title "Carbon-Supported Pseudo-Core–Shell Pd–Pt Nanoparticles for ORR with and without Methanol" @default.
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- W2016058138 doi "https://doi.org/10.1149/1.2926609" @default.
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