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- W2016081021 abstract "Abstract The absorption spectrum of the ν 6 band of C 2 H 3 D centered near 1125.27674 cm −1 in the 1100–1250 cm −1 region was recorded with an unapodized resolution of 0.0063 cm −1 using a Fourier transform infrared (FTIR) spectrometer. A total of 947 infrared transitions of the A – B hybrid-type band were assigned and fitted to upper-state ( ν 6 = 1) rovibrational constants using a Watson’s A -reduced Hamiltonian in the I r representation up to eighth-order centrifugal distortion terms. The b -type infrared transitions of the band were analyzed for the first time. The root-mean-square deviation of the fit was 0.00062 cm −1 . The ground-state rovibrational constants up to eighth-order terms were also obtained by a fit of 617 combination differences from the present infrared measurements, simultaneously with 21 microwave frequencies with a root-mean-square deviation of 0.00055 cm −1 . From this work, the upper-state ( ν 6 = 1) and ground-state constants of C 2 H 3 D were derived with the highest accuracy, so far. The a - and b -type transitions of the hybrid ν 6 band were found to be relatively free from local frequency perturbations. The ratio of the a - to b -type vibrational dipole transition moments ( μ a / μ b ) was found to be 1.05 ± 0.10. From the ν 6 = 1 rovibrational constants obtained, the inertial defect Δ 6 was calculated to be 0.3570 ± 0.0008 μA 2 ." @default.
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- W2016081021 date "2010-10-01" @default.
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- W2016081021 title "The high-resolution FTIR spectrum of the ν6 band of C2H3D" @default.
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- W2016081021 doi "https://doi.org/10.1016/j.jms.2010.08.002" @default.
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