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• W2016099451 abstract "Abstract Chemical-looping combustion (CLC) is very promising with thanks to its efficient and low cost CO 2 capture. For calcium sulfate (CaSO 4 ) oxygen carrier, sulfur dioxide (SO 2 ) emission in CLC process limits its practical application. In this study, Fe 2 O 3 /CaSO 4 composite oxygen carriers with different Fe 2 O 3 loading contents were prepared using impregnation method with natural anhydrite as active support and Fe 2 O 3 as additive. Experiments on the evaluation of their capacities to inhibit SO 2 release and enhance the reactivity of CaSO 4 were conducted in a laboratory scale fixed-bed reactor under CO–H 2 –N 2 atmosphere. The effects of temperature and Fe 2 O 3 loading content on the performance of Fe 2 O 3 /CaSO 4 oxygen carriers were investigated in terms of fuel conversion and sulfur inhibition efficiency. Fe 2 O 3 could intensify the reduction of CaSO 4 to CaS and raise the calcium sulfide yield, over 85% SO 2 released from the decomposition of CaSO 4 alone was inhibited by Fe 2 O 3 /CaSO 4 oxygen carriers with the Fe 2 O 3 loading content higher than 5 wt% at 950 °C. Temperature and Fe 2 O 3 loading content had pronounced positive effect on the reactivity enhancement of CaSO 4 , with higher conversion of CO and H 2 obtained at higher temperature and Fe 2 O 3 loading content. Redox cyclic tests showed that Fe 2 O 3 /CaSO 4 oxygen carrier could keep a better recyclability and stability than CaSO 4 . The higher the Fe 2 O 3 loading content, the higher the reactivity and sulfur inhibition ability Fe 2 O 3 /CaSO 4 oxygen carriers could possess. Overall, the results show that Fe 2 O 3 /CaSO 4 oxygen carrier displays its promising aspect and could be a good candidate in CLC." @default.
• W2016099451 created "2016-06-24" @default.
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• W2016099451 date "2013-09-01" @default.
• W2016099451 modified "2023-09-24" @default.
• W2016099451 title "Performance of Fe2O3/CaSO4 composite oxygen carrier on inhibition of sulfur release in calcium-based chemical looping combustion" @default.
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• W2016099451 doi "https://doi.org/10.1016/j.ijggc.2013.04.010" @default.
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