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• W2016166735 startingPage "358" @default.
• W2016166735 abstract "Summarized here are our continuous studies of the last three decades concerning syntheses of new types of complexes learned from nitrogenase and their reactivites toward dinitrogen, nitriles, and alkynes. For Mo and W dinitrogen complexes with tertiary phosphine coligands, a variety of their intriguing reactivities have been demonstrated, and novel transformations of the N 2 ligands into numerous nitrogen-containing ligands and compounds have been developed. The C≡N bond cleavage of certain nitriles also proceeds on the Mo site surrounded by tertiary phosphines. Stimulated by the sophisticated structure of the active site of nitrogenase, multinuclear metal–sulfur complexes have been synthesized in rational ways. New types of stoichiometric and catalytic reactions of alkynes have been found by using the thiolato-bridged diruthenium complexes and some cubane-type sulfido clusters containing a noble metal.Key words: nitrogen fixation, molybdenum and tungsten dinitrogen complexes, ruthenium thiolato complexes, metal sulfido clusters, nitriles, alkynes." @default.
• W2016166735 created "2016-06-24" @default.
• W2016166735 creator A5017560208 @default.
• W2016166735 creator A5076833319 @default.
• W2016166735 date "2005-04-01" @default.
• W2016166735 modified "2023-09-24" @default.
• W2016166735 title "Research inspired by the chemistry of nitrogenase — Novel metal complexes and their reactivity toward dinitrogen, nitriles, and alkynes" @default.
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• W2016166735 doi "https://doi.org/10.1139/v05-016" @default.
• W2016166735 hasPublicationYear "2005" @default.
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