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• W2016203761 abstract "An ISES (in situ enzymatic screening) lead pointed to conditions (PMP N-protecting group, Ni(cod)2 catalyst precursor) under which chiral, bidentate phosphines could promote Ni(0)-mediated allylic amination. Therefore, bidentate phosphines bearing central, axial, and planar chirality were examined with two model substrates of interest for PLP-enzyme inhibitor synthesis. In the best case, with (R)-MeO-BIPHEP, vinylglycinol derivative 2 was obtained in 75% ee (97% ee, one recrystallization) from 1. Further manipulation provided a Ni(0)-mediated entry into l-vinylglycine." @default.
• W2016203761 created "2016-06-24" @default.
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• W2016203761 date "2004-07-10" @default.
• W2016203761 modified "2023-09-24" @default.
• W2016203761 title "Following an ISES Lead: The First Examples of Asymmetric Ni(0)-Mediated Allylic Amination" @default.
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• W2016203761 doi "https://doi.org/10.1021/ol049159x" @default.
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