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• W2016209150 abstract "The effect of the picrate (pic-) ion on Eu(III) extraction with a diamide (da) from aqueous nitric acid (0.001—0.1 mol dm-3) solutions into benzene was clarified on the basis of the stoichiometry of ion-pair extractions by analyzing the distribution data of Eu(III) and picric acid (Hpic). The extraction of Eu(III) with da was extremely enhanced by adding a hydrophobic anion of pic- to the liquid-liquid system. From analyses of the distribution data of Eu(III) and Hpic, it was concluded that the effect of the hydrophobic anion was caused by the extraction of a single ion-pair of [Eu(da)2](pic)3. The nitrate ion had no relation with the cooperative effect of da and pic-, i.e., the extraction of [Eu(da)2](NO3)3, [Eu(da)2](pic)(NO3)2, and [Eu(da)2](pic)2(NO3) was practically negligible as against the [Eu(da)2](pic)3 extraction. The cooperative effect was reduced by an increase in the aqueous HNO3 concentration, which was induced by a decrease in the pic- concentration in the aqueous phase; the dissociation of Hpic into pic- ion was suppressed by an increase in the H+ concentration, and a part of molecular Hpic was extracted into the organic phase. Furthermore, the extraction of Hpic was also enhanced by an increase in the da concentration in the organic phase, which also induced a decrease in the aqueous pic- concentration. This was found to be due to the formation of a 1 : 1 complex between da and Hpic. However, the extraction of the complexes between da and HNO3 was negligible in the acid concentration range in the present study." @default.
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• W2016209150 date "2000-03-01" @default.
• W2016209150 modified "2023-09-27" @default.
• W2016209150 title "Effect of the Hydrophobic Anion of Picrate on the Extraction of Europium(III) with Diamide" @default.
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• W2016209150 doi "https://doi.org/10.1246/bcsj.73.623" @default.
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