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- W2016243767 abstract "Recent work has emphasized that the rebinding kinetics of ligands to heme systems can exhibit nonexponential kinetics below the glass transition due to inhomogeneous spreads in factors other than enthalpy. We show that an expected distribution in the nonadiabatic electronic prefactor will lead to a t−1/2 dependence for the rebinding rate at long times. This will occur at temperatures below the glass transition but for T≳1/2αR, where α characterizes the enthalpy spread and R is the gas constant. We show that this spread in prefactor explains the long time behavior in the appropriate temperature range for Mb–CO and Mb3–CO." @default.
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- W2016243767 modified "2023-10-18" @default.
- W2016243767 title "Control of long time dependence of CO binding to heme systems by inhomogeneous spread in electronic prefactor" @default.
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- W2016243767 doi "https://doi.org/10.1063/1.468909" @default.
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