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• W2016348300 abstract "Photoionization and photodissociation of ferrocene [Fe(C5H5)2] is examined by using vacuum ultraviolet (VUV) photons from a synchrotron radiation source and a time-of-flight (TOF) photoionization mass spectrometer. VUV absorption by ferrocene results in Fe(C5H5)2·+, FeC5H5+, FeC3H3+, Fe·+ and C10Hx·+ (x = 8 − 10). The dependency of the product distribution on photon energy indicates sequential elimination of C5H5· ligands as a major dissociation channel, but concerted elimination of two C5H5· ligands also takes place to a lesser degree. Through analysis of TOF peak shape, it is found that Fe(C5H5)2·+ molecular ion dissociates into FeC5H5+ and C5H5· via two channels. One is nonstatistical dissociation with a fast rate, and the other is slow unimolecular decay that becomes more discernible at low photon energy. The rate of unimolecular decay, exemplified by a value of k = 2.4 ± 1.0 × 106 s−1 at photon energy of 14.76 eV, is well in accord with the RRKM rate." @default.
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• W2016348300 date "1998-12-01" @default.
• W2016348300 modified "2023-10-12" @default.
• W2016348300 title "Vacuum ultraviolet photoionization and photodissociation of ferrocene" @default.
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• W2016348300 doi "https://doi.org/10.1016/s1387-3806(98)14176-3" @default.
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