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- W2016356943 abstract "The structural transformation from a discrete cluster to a wave-like chain played by the pz molecules. Two new Keggin polyoxometalate-based compounds, [Ag 4 (phnz) 6 (SiW 12 O 40 )] (phnz = phenazine) ( 1 ) and [Ag(phnz) 1.5 ][Ag(phnz)(pz)][{Ag 2 (phnz)(pz)(H 2 O)}(SiW 12 O 40 )] ( 2 ) (pz = pyrazine), have been hydrothermally synthesized. Compound 1 is a discrete cluster in which the [SiW 12 O 40 ] 4− (SiW 12 ) anion symmetrically connects two dinuclear Ag 2 (phnz) 3 fragments. All Ag I in 1 adopt a trigonal geometry. By introducing the secondary bridging ligand “pz” into the above system, compound 2 was obtained. Compound 2 contains three kinds of silver complex subunits: [Ag 2 (phnz)(pz)(H 2 O)] 2+ , [Ag 2 (phnz) 3 ] 2+ and [Ag(phnz)(pz)] + . The first one extends to a wave-like chain with SiW 12 anions as bi-dentate suspenders, and the last two are counter cations. Furthermore, Ag I ions in 2 exhibit three kinds of coordination modes. Their electrochemistry properties have also been studied." @default.
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- W2016356943 date "2010-11-01" @default.
- W2016356943 modified "2023-10-16" @default.
- W2016356943 title "Two new polyoxometalate-based hybrids: Structural transformation played by a secondary bridging ligand" @default.
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- W2016356943 doi "https://doi.org/10.1016/j.ica.2010.07.027" @default.
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