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• W2016376945 abstract "A molecular dynamics simulation (MD) of a generic model for polymers adsorbed on a discrete surface is presented. We investigate the effect of surface roughness on the film's diffusion constant, its influence on aging, and other properties. The model reproduces many experimentally observed features such as logarithmic aging of structural properties with time, a power law aging of the diffusion constant D, and the anomalous dependence of mobility with surface coverage. It is shown that the glassy dynamics is intimately linked to the roughness, which can be controlled by changing the interaction potential between surface atoms and adsorbed particles. We observe a logarithmic increase in the structure factor with aging time and a power law decay in D only if the corrugation is sufficiently high. For a smooth surface, no such time dependence is observed, even if adhesion and thus confinement is increased. We also address the question as to why the mobility of adsorbed polymers can initially increase with surface coverage Γ when Γ is low." @default.
• W2016376945 created "2016-06-24" @default.
• W2016376945 creator A5056117766 @default.
• W2016376945 creator A5083960327 @default.
• W2016376945 date "2007-02-10" @default.
• W2016376945 modified "2023-09-27" @default.
• W2016376945 title "Glassy Dynamics, Aging in Mobility, and Structural Relaxation of Strongly Adsorbed Polymer Films: Corrugation or Confinement?" @default.
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• W2016376945 doi "https://doi.org/10.1021/ma0627370" @default.
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