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• W2016450489 abstract "By using x-ray absorption spectroscopy at the $text{Rh}text{ }{L}_{2,3}$, $text{Co}text{ }{L}_{2,3}$, and $text{Fe}text{ }{L}_{2,3}$ edges, we find a valence state of ${text{Co}}^{2+}/{text{Rh}}^{4+}$ in ${text{Ca}}_{3}{text{CoRhO}}_{6}$ and of ${text{Fe}}^{3+}/{text{Rh}}^{3+}$ in ${text{Ca}}_{3}{text{FeRhO}}_{6}$. X-ray magnetic circular dichroism spectroscopy at the $text{Co}text{ }{L}_{2,3}$ edge of ${text{Ca}}_{3}{text{CoRhO}}_{6}$ reveals a giant orbital moment of about $1.7{ensuremath{mu}}_{B}$, which can be attributed to the occupation of the minority-spin ${d}_{0}{d}_{2}$ orbital state of the high-spin ${text{Co}}^{2+}$ $(3{d}^{7})$ ions in trigonal prismatic coordination. This active role of the spin-orbit coupling explains the strong magnetocrystalline anisotropy and Ising-type magnetism of ${text{Ca}}_{3}{text{CoRhO}}_{6}$." @default.
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• W2016450489 date "2008-05-14" @default.
• W2016450489 modified "2023-10-18" @default.
• W2016450489 title "X-ray absorption and x-ray magnetic dichroism study on<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:msub><mml:mrow><mml:mtext>Ca</mml:mtext></mml:mrow><mml:mn>3</mml:mn></mml:msub><mml:msub><mml:mrow><mml:mtext>CoRhO</mml:mtext></mml:mrow><mml:mn>6</mml:mn></mml:msub></mml:mrow></mml:math>and<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:msub><mml:mrow><mml:mtext>Ca</mml:mtext></mml:mrow><mml:mn>3</mml:mn></mml…" @default.
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• W2016450489 doi "https://doi.org/10.1103/physrevb.77.205111" @default.
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