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• W2016465596 startingPage "015006" @default.
• W2016465596 abstract "Core@shell and concentration-gradient particles have attracted much attention as improved cathodes for Li-ion batteries (LIBs). However, most of their preparation routes have employed a precisely-controlled co-precipitation method. Here, we report a facile preparation route of core@shell and concentration-gradient spinel particles by dry powder processing. The core@shell particles composed of the MnO2 core and the Li(Ni,Mn)2O4 spinel shell are prepared by mechanical treatment using an attrition-type mill, whereas the concentration-gradient spinel particles with an average composition of LiNi0.32Mn1.68O4 are produced by calcination of their core@shell particles as a precursor. The concentration-gradient LiNi0.32Mn1.68O4 spinel cathode exhibits the high discharge capacity of 135.3 mA h g−1, the wide-range plateau at a high voltage of 4.7 V and the cyclability with a capacity retention of 99.4% after 20 cycles. Thus, the facile preparation route of the core@shell and concentration-gradient particles may provide a new opportunity for the discovery and investigation of functional materials as well as for the cathode materials for LIBs." @default.
• W2016465596 created "2016-06-24" @default.
• W2016465596 creator A5016709273 @default.
• W2016465596 creator A5089058595 @default.
• W2016465596 date "2015-02-25" @default.
• W2016465596 modified "2023-10-18" @default.
• W2016465596 title "Facile preparation of core@shell and concentration-gradient spinel particles for Li-ion battery cathode materials" @default.
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• W2016465596 doi "https://doi.org/10.1088/1468-6996/16/1/015006" @default.
• W2016465596 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/5036501" @default.
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