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- W2016507716 abstract "We have studied the glass transition temperature (${T}_{g}$) and molecular mobility of polystyrene (PS) thin films near the interface between the polymer thin film and substrate with bilayer thin films consisting of surface hydrogenated PS (h-PS) and bottom deuterated PS (d-PS) using neutron reflectivity. With decreasing the thickness of the bottom d-PS layer, ${T}_{g}$ near the interface between the polymer thin film and substrate increased compared to bulk ${T}_{g}$ and a drastic increase of ${T}_{g}$ was observed for the bottom d-PS layer 155 AA{} thick. The orientation of polymer chains at the interface is supposed to be related to the increase of ${T}_{g}$ near the interface between the polymer and substrate. The polymer chain mobility decreased with thickness even for the bottom d-PS layer with no discernible change of ${T}_{g}$. It is considered that the numerous contacts between polymer chains and substrate are related to the decrease of mobility near the interface between the polymer thin film and substrate." @default.
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- W2016507716 date "2011-09-16" @default.
- W2016507716 modified "2023-10-07" @default.
- W2016507716 title "Interfacial properties of polystyrene thin films as revealed by neutron reflectivity" @default.
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- W2016507716 doi "https://doi.org/10.1103/physreve.84.031802" @default.
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