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• W2016575450 abstract "Femtosecond laser pulse irradiation of inorganic glasses allows a selective modification of the optical properties withvery high precision. This results in the possibility for the production of three-dimensional functional optical elements inthe interior of glass materials, such as optical data storage, waveguide writing, etc. The influence of the chemical glasscomposition to the response upon ultrashort laser irradiation has not been studied systematically. For that, simple silicabasedmodel glasses composed of systematically varying alkaline- and earth-alkaline components were prepared,irradiated on the surface and in the volume with single fs-laser pulses (~130 fs, 800 nm), and were subsequentlyanalyzed by means of micro-Raman spectroscopy and quantitative phase contrast microscopy in order to account forchanges in the glass structure and for alterations of the optical refractive index, respectively. The Raman spectroscopicstudies of the laser-irradiated spots revealed no change in the average binding configuration (the so called Q-structure),but local changes of bond-angles and bond-lengths within the glass structure structure. Those changes are explained bystructural relaxation of the glass network due to densification caused by a transient laser-induced plasma generation andthe following shock wave and other thermal phenomena. Glasses with a low amount of network modifiers show changesin the Si-O network while glasses with a high amount of network modifiers react primarily via variation of the nonbridgingoxygen ions. The results are discussed in terms of possible structural response mechanisms and conclusions areoutlined regarding glass compositions with technical suitability for fs-laser modifications." @default.
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• W2016575450 date "2013-11-14" @default.
• W2016575450 modified "2023-10-03" @default.
• W2016575450 title "Compositional dependent response of silica-based glasses to femtosecond laser pulse irradiation" @default.
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• W2016575450 doi "https://doi.org/10.1117/12.2028713" @default.
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