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- W2016598560 abstract "Abstract Carbon single‐wall nanotubes (SWNTs) were loaded with 5.4 wt.% H by exposing to a hydrogen pressure of 50 kbar at 500°C. Investigation of the optical transmission spectra showed that the hydrogenation significantly suppressed the high‐frequency conductivity σ of free carries in the SWNTs and also eliminated the band‐to‐band electronic transitions. Instead, a narrow line of the C‐H stretching vibrational mode appeared at 2845 cm−1. A gradual removal of hydrogen from the hydrogenated SWNTs by vacuum annealing at T≥500°C resulted in an approximately linear decrease in the intensity of this line with decreasing hydrogen content. This evidenced that most H atoms in the hydrogenated SWNTs were covalently bonded to the carbon atoms. The complete removal of hydrogen by vacuum annealing at 700°C partly restored σ and the intensity of the electronic transitions characteristic of the initial SWNTs." @default.
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- W2016598560 date "2006-12-01" @default.
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- W2016598560 title "Electronic and Vibration Spectra of Hydrogenated Carbon Single‐Wall Nanotubes" @default.
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- W2016598560 doi "https://doi.org/10.1080/15363830600663487" @default.
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