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- W2016658105 abstract "Nucleation and condensation processes are investigated in finite systems by means of the Helmholtz free energy of formation of microclusters. The radius of clusters and the number of clusters are related to each other in such a system. A maximum of the free energy i.e., the critical state and a minimum i.e., the metastable state are found to be dependent on the number of microclusters present in the system. For a given number of particles (i.e., supersaturation) a maximum number of clusters exists. In this state the maximum and the minimum of the free energy are equal. This condition defines the first metastable state of the system. Condensation may start at this point and proceed along a line in the “valley” of the free energy until the equilibrium between bulk liquid and vapor is reached. Kinetic equations are derived for the condensation process using this thermodynamic concept. The relations obtained differ significantly from the classical ones. Data for water vapor condensation from the literature are used to test the validity of the theory presented. Sufficient agreement is found. The present theory appears to correlate condensation experiments obtained by different techniques." @default.
- W2016658105 created "2016-06-24" @default.
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- W2016658105 date "1982-07-01" @default.
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- W2016658105 title "Thermodynamics of finite systems: a possibility for interpretation of nucleation and condensation experiments" @default.
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- W2016658105 doi "https://doi.org/10.1016/0021-9797(82)90151-5" @default.
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