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- W2016704489 abstract "Abstract The molybdenum purple bronze KMo 6 O 17 is quasi two-dimensional (2D) metallic oxide that shows a Peierls transition towards a metallic charge density wave state. Since this specific transition is directly related to the electron properties of the normal state, we have investigated the electronic structure of this bronze at room temperature. The shape of the Mo K1s absorption edge reveals the presence of distorted MoO 6 octahedra in the crystallographic structure. Photoemission experiments evidence a large conduction band, with a bandwidth of 800 meV and confirm the metallic character of this bronze. A wide depleted zone separates the conduction band from the valence band that exhibits a fourfold structure, directly connected to the octahedral symmetry of the Mo sites. The band structure is determined by ARUPS in two main directions of the (0 0 1) Brillouin zone. It exhibits some unpredicted features but corroborates the earlier theoretical band structure and Fermi surface. It confirms the hidden one-dimensionality of KMo 6 O 17 that has been proposed to explain the origin of the Peierls transition in this 2D compound." @default.
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- W2016704489 date "2006-09-01" @default.
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- W2016704489 title "Band structure of the quasi two-dimensional purple molybdenum bronze" @default.
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- W2016704489 doi "https://doi.org/10.1016/j.susc.2005.12.075" @default.
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