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• W2016708595 abstract "We propose an accurate method to predict interfacial tension between water and nonpolar fluids by using Cahn gradient theory. The only necessary elements are (i) a water contact energy function and (ii) an equation of state (EoS) for the nonpolar fluid, chosen here as the Peng−Robinson EoS. The contact energy, a function of the fluid (adsorbate) surface density, is related to interfacial tension (IFT) by means of the Gibbs adsorption equation. Examining a large number of IFT data, we observe that the water contact energy is a universal function of adsorbate's surface density when proper scaling variables are used: it depends neither on adsorbate nor on temperature. A corresponding-states principle appears to govern the interfacial behavior between water and any nonpolar compound that is sparingly soluble in water. A predictive method (without any adjustable parameter) is therefore available for estimating IFT between water and any nonpolar fluid, whether the fluid is in supercritical or in subcritical states. The method performs well when the adsorbate is sparingly soluble in water, but slightly overestimates IFTs when the adsorbate's solubility in water is significant (e.g., CO2 and H2S). A similar behavior should also hold for interfaces involving a solid substrate." @default.
• W2016708595 created "2016-06-24" @default.
• W2016708595 creator A5028343479 @default.
• W2016708595 creator A5065154402 @default.
• W2016708595 date "2007-10-31" @default.
• W2016708595 modified "2023-09-26" @default.
• W2016708595 title "Predicting Interfacial Tension between Water and Nonpolar Fluids from a Cahn-Type Theory" @default.
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• W2016708595 doi "https://doi.org/10.1021/la701893z" @default.
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