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- W2016782190 abstract "Explicit formulas for the excess chemical potential and Helmholtz free energy have been derived in different ways making use of a functional integration technique. The method employed is an extension of the Kirkwood ‘‘charging’’ procedure and involves a new way of renormalizing cluster series. The formulas require only the correlation functions for the system under investigation. New and old ways of calculating the free energy of a simple fluid are compared and discussed. Numerical results for the various closures are presented for hard and Lennard-Jones sphere fluids. A bridge functional of the first kind has been introduced and some approximations for this have been proposed and tested." @default.
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- W2016782190 date "1990-08-01" @default.
- W2016782190 modified "2023-10-14" @default.
- W2016782190 title "Free energy in the statistical theory of fluids" @default.
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- W2016782190 doi "https://doi.org/10.1063/1.459071" @default.
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