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• W2016794669 abstract "We describe a highly efficient, general strategy for the enantioselective synthesis of benzomorphans (45-46% overall yield from commercially available material). The new synthesis demonstrates the effectiveness of an unprecedented diastereoselective cycloisomerization via migratory hydroamination and the power of palladium-catalyzed asymmetric allylic alkylation (AAA) of simple ketone enolates in the context of complex synthesis. The strategy outlined here for the enantioselective synthesis of three contiguous stereogenic centers and the novel cycloisomerization should have many applications in alkaloid synthesis." @default.
• W2016794669 created "2016-06-24" @default.
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• W2016794669 date "2003-06-28" @default.
• W2016794669 modified "2023-10-17" @default.
• W2016794669 title "Migratory Hydroamination: A Facile Enantioselective Synthesis of Benzomorphans" @default.
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• W2016794669 doi "https://doi.org/10.1021/ja0360539" @default.
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