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• W2017025359 abstract "Singlet fission sensitized photovoltaics have the potential to surpass the Shockley-Queisser limit for a single-junction structure. We investigate the dynamics of triplet excitons resulting from singlet fission in pentacene and their ionization at a C60 heterojunction. We model the generation and diffusion of excitons to predict the spectral response. We find the triplet diffusion length in polycrystalline pentacene to be 40 nm. Poly(3-hexylthiophene) between the electrode and pentacene works both to confine triplet excitons and also to transfer photogenerated singlet excitons into pentacene with 30% efficiency. The lower bound for the singlet fission quantum efficiency in pentacene is 180 ± 15%." @default.
• W2017025359 created "2016-06-24" @default.
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• W2017025359 date "2013-10-07" @default.
• W2017025359 modified "2023-10-05" @default.
• W2017025359 title "Triplet diffusion in singlet exciton fission sensitized pentacene solar cells" @default.
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• W2017025359 doi "https://doi.org/10.1063/1.4824420" @default.
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