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- W2017051698 abstract "Control over various fragmentation reactions of a series of polyatomic molecules (acetylene, ethylene, 1,3-butadiene) by the optical waveform of intense few-cycle laser pulses is demonstrated experimentally. We show both experimentally and theoretically that the responsible mechanism is inelastic ionization from inner-valence molecular orbitals by recolliding electron wave packets, whose recollision energy in few-cycle ionizing laser pulses strongly depends on the optical waveform. Our work demonstrates an efficient and selective way of predetermining fragmentation and isomerization reactions in polyatomic molecules on subfemtosecond time scales." @default.
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- W2017051698 date "2012-12-10" @default.
- W2017051698 modified "2023-10-06" @default.
- W2017051698 title "Attosecond-Recollision-Controlled Selective Fragmentation of Polyatomic Molecules" @default.
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- W2017051698 doi "https://doi.org/10.1103/physrevlett.109.243001" @default.
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