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- W2017059504 abstract "A self-consistent integral equation theory is presented for the conformational properties and spinodal lines of random copolymer melts. The theory combines field-theoretic methods with the polymer reference interaction site model (PRISM) theory. The many-chain problem is replaced by a single chain where the sites interact via a bare plus a self-consistently determined medium-induced potential, and the conformational properties are obtained using a variational method. The theoretical prediction for the spinodal line is qualitatively similar to that of non-self-consistent PRISM theory. The theory predicts macroscopic phase separation for all values of the monomer correlation strength, λ. The inverse spinodal temperature is a nonmonotonic function of λ with a maximum at λmax. For large values of λ(≈1), the values of spinodal temperatures are almost identical to those of non-self-consistent PRISM theory. For low values of λ, however, the theory predicts higher values for spinodal temperatures than non-self-consistent PRISM theory. The theory predicts significant changes in the mean-square end-to-end distance as the temperature is decreased." @default.
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- W2017059504 date "2005-06-15" @default.
- W2017059504 modified "2023-10-17" @default.
- W2017059504 title "Integral equation theory of random copolymer melts: Self-consistent treatment of intramolecular and intermolecular correlations" @default.
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- W2017059504 doi "https://doi.org/10.1063/1.1931649" @default.
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