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- W2017111962 abstract "Abstract Summary: This paper presents the synthesis of two polymeric surfactants, consisting of a polysiloxane backbone with amphiphilic side chains of the nonionic oligo(ethylene oxide) type, and their phase behavior in aqueous solution, investigated by polarizing microscopy and deuterium NMR spectroscopy using D 2 O as a probe. Two different side chains, which are isomeric glycerol derivatives, were synthesized and attached to poly(methyl hydrogen siloxane) by a hydrosilylation reaction, resulting in a tail‐type and a mid‐type polysurfactant. The side chains of the tail‐type system are fixed at the end of the hydrophobic moiety, whereas the side‐chains of the mid‐type system are tethered to the polymer backbone by a short spacer close to the hydrophilic‐hydrophobic junction of the amphiphile. Both polymers form a lamellar phase in aqueous solution over a wide range of concentrations, whereas the side chain precursors do not form lyomesophases. The cloud curve and the lamellar region are observed at lower temperatures in the mid‐type polysurfactant. Structures of the isomeric polymers forming lamellar phases. magnified image Structures of the isomeric polymers forming lamellar phases." @default.
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- W2017111962 date "2006-02-08" @default.
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- W2017111962 title "Lyotropic Lamellar Polysiloxanes with Isomeric Amphiphilic Side Chains" @default.
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- W2017111962 doi "https://doi.org/10.1002/macp.200500452" @default.
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