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W2017180582 abstract "Abstract As an alternative to the Fickian model of solute diffusion-sorption in matrices of geological media, a first-order kinetic model with diffusion-equivalent rate parameters was developed using temporal moment analysis of breakthrough curves for a parallel fracture system, hollow cylindrical macropores, and cylindrical solid phase. Criteria on the difference between the breakthrough curves of the Fickian model and the first-order kinetic model were also derived through temporal moment analysis. The criterion for the parallel fracture system was examined in detail to determine the validity of a first-order kinetic model approximation in in-situ rock fracture systems. The accuracy of the approximation was greater for smaller fracture spacings, longer groundwater residence time, and larger matrix diffusion coefficients, but was independent of nuclide distribution coefficients. Existence of natural rock-fracture systems to which the kinetic model approximation can be applied was shown to be possible." @default.
W2017180582 created "2016-06-24" @default.
W2017180582 creator A5081822811 @default.
W2017180582 creator A5088598116 @default.
W2017180582 date "1993-05-01" @default.
W2017180582 modified "2023-09-22" @default.
W2017180582 title "Application of a simple model for assessment of underground radionuclide migration. Part I. Validity of first-order kinetic model approximation" @default.
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W2017180582 doi "https://doi.org/10.1016/0022-1694(93)90223-v" @default.
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