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• W2017226054 abstract "The Daphniphyllum alkaloids are a group of highly complex polycyclic alkaloids. Examination of the structures if several members of this family of natural products led to a hypothesis about their mode of biosynthesis (depicted in Scheme SI ). Based on this hypothetical biosynthetic pathway, a laboratory synthesis was designed that incorporated as a key transformation the novel one-pot transformation of dialdehyde 24 to pentacyclic unsaturated amine 25. This process turned out to be an exceptionally efficient way to construct the pentacyclic nucleus of the Daphniphyllum alkaloids. However, a purely fortuitous discovery, resulting from accidental use of methylamine rather than ammonia, led to a great improvement in the synthesis and suggests an even more attractive possible biosynthesis." @default.
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• W2017226054 date "1996-12-10" @default.
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• W2017226054 title "Nature knows best: An amazing reaction cascade is uncovered by design and discovery" @default.
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• W2017226054 doi "https://doi.org/10.1073/pnas.93.25.14323" @default.
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