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• W2017232207 abstract "Aggregate formation in molecular solids usually quenches the luminescence, a piece of bad news for molecular electronic devices. However, siloles present extremely high luminescent efficiency in solid state as well as in aggregation, but have almost no luminescence in solution. By employing a first-principles calculation to study excited states and vibronic couplings, we find that it is the low-frequency twisting motions of side rings which enhance the nonradiative decay. These motions can be suppressed either by solid-state packing, by aggregation formation in polar solvents, or by increasing the solvent viscosity; thereby, the radiative decay becomes dominant, resulting in peculiar aggregate-induced emission phenomena in siloles." @default.
• W2017232207 created "2016-06-24" @default.
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• W2017232207 date "2006-05-12" @default.
• W2017232207 modified "2023-10-01" @default.
• W2017232207 title "Aggregation-enhanced luminescence and vibronic coupling of silole molecules from first principles" @default.
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• W2017232207 doi "https://doi.org/10.1103/physrevb.73.205409" @default.
• W2017232207 hasPublicationYear "2006" @default.
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