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• W2017272690 abstract "Langmuir–Blodgett films (LB) of arachidic acid (AA, CH3(CH2)18COOH) at the glass/air interface are investigated by sum-frequency generation (SFG) vibrational spectroscopy for all the possible polarization combination of input and output radiation. The newly identified band at 2818 cm−1 in LB films has been attributed to a soft mode of the CH vibration induced by the interaction (coupling) with the rest of molecules near the glass substrate. The coherent response of the CH3-stretching vibration in LB films and self-assembled monolayer (SAM) films of octadecanethiol on gold are also studied as a function of the delay between the visible and infrared radiation, i.e. the free-induction delay (FID). The pure dephasing time T2* obtained for the first time for the LB film is ∼3.2 ps, which is fairly long, reflecting the methyl group coupled with the rest of the molecules near the glass substrate. The short dephasing time of ∼1.0 ps obtained for the SAM film mainly represents the relaxation time of the lattice phonon of gold film." @default.
• W2017272690 created "2016-06-24" @default.
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• W2017272690 date "2005-05-01" @default.
• W2017272690 modified "2023-10-16" @default.
• W2017272690 title "Sum-frequency generation of the symmetric CH3-stretching vibration in organized molecular ultrathin films: ultrafast coupling interaction effect" @default.
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• W2017272690 doi "https://doi.org/10.1016/j.colsurfa.2004.10.084" @default.
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