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• W2017290068 abstract "The influence of water vapor on the production of nitric acid in the gas-phase HO(2) + NO reaction was determined at 298 K and 200 Torr using a high-pressure turbulent flow reactor coupled with a chemical ionization mass spectrometer. The yield of HNO(3) was found to increase linearly with the increase of water concentration reaching an enhancement factor of about 8 at [H(2)O] = 4 x 10(17) molecules cm(-3) ( approximately 50% relative humidity). A rate constant value k(1bw) = 6 x 10(-13) cm(3) molecule(-1) s(-1) was derived for the reaction involving the HO(2)xH(2)O complex: HO(2)xH(2)O + NO --> HNO(3) (1bw), assuming that the water enhancement is due to this reaction. k(1bw) is approximately 40 times higher than the rate constant of the reaction HO(2) + NO --> HNO(3) (1b), at the same temperature and pressure. The experimental findings are corroborated by density functional theory (DFT) calculations performed on the H(2)O/HO(2)/NO system. The significance of this result for atmospheric chemistry and chemical amplifier instruments is briefly discussed. An appendix containing a detailed consideration of the possible contribution from the surface reactions in our previous studies of the title reaction and in the present one is included." @default.
• W2017290068 created "2016-06-24" @default.
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• W2017290068 date "2009-09-28" @default.
• W2017290068 modified "2023-09-25" @default.
• W2017290068 title "Water Vapor Effect on the HNO₃ Yield in the HO₂ + NO Reaction: Experimental and Theoretical Evidence" @default.
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• W2017290068 doi "https://doi.org/10.1021/jp811428p" @default.
• W2017290068 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/19780600" @default.
• W2017290068 hasPublicationYear "2009" @default.
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