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- W2017314897 abstract "This paper describes the steady-state chemical performance of catalytic surfaces of similar constitution but of varied global curvature exposed to two distinct chemical species which are allowed to adsorb, desorb, diffuse and react on the surface. The surface reactions are modeled to include the presence of defect structures which exist due to lattice faults and/or foreign material on the surface. Flat, circular and elliptical cylindrical surfaces are examined with similar desorption and reaction rates at the defect sites so as to evaluate the role of surface curvature on the steady-state behavior of the surface species concentrations. The methodology described here is applicable to generally curved surfaces referred to general curvilinear coordinates generated numerically to conform with the surface shapes. The continuum reaction–diffusion models transformed to the general curvilinear coordinates are solved numerically by the line successive-over-relaxation (SOR) method. Numerical results show that decreasing the surface curvature enhances the chemical process in the presence of surface defects. © 2002 Elsevier Science B.V. All rights reserved." @default.
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- W2017314897 date "2002-01-01" @default.
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- W2017314897 title "Effect of catalytic surface curvature on the chemical performance with defect structures" @default.
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- W2017314897 doi "https://doi.org/10.1016/s1385-8947(01)00139-5" @default.
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