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- W2017372000 abstract "Two-dimensional interfacial electrodeposition of silver is studied under alternating square-wave electric potential conditions, at the water/dichloromethane interface. The overall rate of growth is found to increase with frequency. The deposit's morphology also depends strongly on the frequency: at ≤10 Hz compact deposits are formed while at 1−10 kHz highly ramified structures develop, the branches in which tend to broaden out at higher frequencies. At ∼100 Hz a highly disordered growth is observed. A novel pulsating behavior of the deposit size is observed, with alternating contractions and growth phases. The contractions are attributed to a mechanical compaction of the newly-formed deposit, driven by the fast changes in surface tension due to the voltage variation. The mechanical oscillations induce hydrodynamic stirring in the solution, affecting the mass-transport of the reacting silver ions to the electrode, and, consequently, the rate of growth and morphology of the deposit." @default.
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- W2017372000 date "1997-08-01" @default.
- W2017372000 modified "2023-09-23" @default.
- W2017372000 title "AC-Driven Interfacial Electrodeposition of Silver" @default.
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- W2017372000 doi "https://doi.org/10.1021/la970064w" @default.
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