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• W2017413352 abstract "A systematic investigation of the electrochemical oxidation of copper cyanide was carried out. At low pH, cyanide destruction is believed to be catalyzed by the heterogeneous reaction involving adsorbed [Cu(CN)3]2− and possibly [Cu(CN)4]3−. At high pH, rapid oxidation of cyanide was observed around 0.75 V versus Hg/HgO with the formation of a black copper oxide film. This enhanced electrocatalytic activity is believed to be related to the formation of an active copper(III) species. The transition point between low and high pH as a function of cyanide and copper concentrations is discussed. Bulk electrolysis of a copper cyanide solution at 0.90 V oxidized most of the cyanide to cyanate. Prolonged electrolysis further oxidized the cyanate to nitrate. The copper oxide film is found to be catalytic, capable of electro-oxidizing hydroxide to oxygen and cyanate to nitrate." @default.
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• W2017413352 date "2002-08-01" @default.
• W2017413352 modified "2023-09-27" @default.
• W2017413352 title "The electrochemical oxidation of alkaline copper cyanide solutions" @default.
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• W2017413352 doi "https://doi.org/10.1016/s0013-4686(02)00200-1" @default.
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