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- W2017448704 abstract "Separation of Cs and Sr from simulated high-level radioactive liquid waste (HLLW) was performed using an octylphenyl-N,N-diisobutylcarbomoyl phosphine oxide impregnated silica adsorbent (CMPO-adsorbent). As part of HLLW treatment, the adsorbent is subjected to strong irradiation. Therefore, the durability of CMPO-adsorbent under gamma-ray irradiation conditions was studied. CMPO decomposed to phosphoric acid after a transition to octylphenyl phosphinic acid (OPP). The adsorbed amount of actinoids and lanthanoids were found to decrease linearly with increasing irradiation dose. However, at a dose of 2 MGy, the CMPO-adsorbent was able to maintain adsorption at a rate of 80% of its initial capacity. Based on this finding, it is estimated that the adsorbent can be used in the treatment of HLLW for 400-500 cycles. Radiolytic degradation products increase with increasing irradiation dose caused by HLLW. If OPP accumulates in a CMPO-adsorbent, actinoids and lanthanoids are not recovered. OPP dissolves easily by washing with an eluent, suggesting that OPP would not accumulate in the adsorbent. After washing, separation performance was maintained with a dose of 2 MGy." @default.
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- W2017448704 date "2006-05-01" @default.
- W2017448704 modified "2023-09-25" @default.
- W2017448704 title "Durability of CMPO Impregnated Silica Adsorbent under Irradiation Conditions" @default.
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- W2017448704 doi "https://doi.org/10.1080/18811248.2006.9711134" @default.
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