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• W2017455693 abstract "The infrared dielectric property of monoclinic BaTeMo2O9 single crystals is studied by polarized IR reflectance spectra from 20 to 1800 cm−1. Based on the modified Lorentz model, the frequencies, strengths, and dampings of TO modes as well as the orientations of the dipole momenta are determined, agreeing well with Raman spectra and results from First-principles calculation. The observed modes are visually assigned to the specific atoms' motions in the primitive cell based on the theory calculations. A large shift of the internal modes of the anion groups relative to free anion co-ordination polyhedra is observed, which can be used to indicate the distortions of co-ordination polyhedra related to the nonlinear optical properties. Further, the experimental results of the strengths of the oscillators support the elimination and splitting of degenerate modes in free regular polyhedrons. These results offer a way to evaluate the nonlinear optical properties by use of traditional IR reflectivity spectra." @default.
• W2017455693 created "2016-06-24" @default.
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• W2017455693 date "2013-12-17" @default.
• W2017455693 modified "2023-10-14" @default.
• W2017455693 title "Effects of structure distortion on optical phonon properties of crystalline beta-BaTeMo2O9—A novel nonlinear optical material: Infrared and Raman spectra as well as first-principles calculations" @default.
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• W2017455693 doi "https://doi.org/10.1063/1.4844555" @default.
• W2017455693 hasPublicationYear "2013" @default.
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